"In order to explain the phenomena of radio-activity, a theory has been put forward which regards the atoms of the radio-active elements as suffering spontaneous disintegration, and giving rise to a series of radio-active substances which differ in chemical properties from the parent elements. The radiations accompany the breaking-up of the atoms, and afford a comparative measure of the rate at which the disintegration takes place. This theory is found to account in a satisfactory way for all the known facts of radio-activity, and welds a mass of disconnected facts into one homogeneous whole."
January 1, 1970
https://en.wikiquote.org/wiki/Radio-activity